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Second harmonic generation (SHG) using intense Hermite-Gaussian laser beam (HGLB) propagating through the plasma for mode-indices m = 0 and m = 1 is reported in the present work. Ponderomotive force induced density perturbation beats with the oscillatory velocity of electrons at incident laser frequency, generate the second harmonic nonlinear current that give rise to SHG. Using paraxial approximations, we have derived the coupled equations for the beam width parameter of HGLB and second harmonic's normalized amplitude. Resonance condition is obtained by considering wiggler magnetic field which providing an extra momentum to the second harmonic photon and this result a significant increase in the amplitude of SHG. Our analysis shows the prominent rise in normalized amplitude of second harmonic on increasing the value of the intensity of fundamental laser pulse, normalized wiggler magnetic field and normalized density of plasma. It is notified that the gain of SHG is more prominent for m = 1. Dependency of laser and plasma parameters on SHG is also reported in the current work. 相似文献
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Zihua Guo Xingxing Liu Luc Molinet Zhaoyang Yin 《Journal of Differential Equations》2019,266(2-3):1698-1707
We prove norm inflation and hence ill-posedness for a class of shallow water wave equations, such as the Camassa–Holm equation, Degasperis–Procesi equation and Novikov equation etc., in the critical Sobolev space and even in the Besov space for . Our results cover both real-line and torus cases (only real-line case for Novikov), solving an open problem left in the previous works ([5], [14], [16]). 相似文献
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Yuzhi Xu Yanfei Zhang Huihui Yang Wen Yin Leli Zeng Shuo Fang Si-Yang Liu Zong Dai Xiaoyong Zou Yihang Pan 《中国化学快报》2022,33(2):968-972
A reliable and sensitive strategy which can assess nucleic acid levels in living cells would be essential for fundamental research of biomedical applications. Some nanomaterial-based fluorescence biosensors recently developed for detecting nucleic acids, however, are often with expensive, complicated and timeconsuming preparation process. Here, by using a facile bottom-up synthesis method, a two-dimensional(2 D) coordination polymer(CP) nanosheet, [Cu(tz)](Htz = 1,2,4-triazole), was successfully... 相似文献
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Zhipeng Lin Hao Zhang Guofeng Liang Yanqi Jin Hongbin Zeng Jiawang Li Jian Chen Weihong Zhang Fangyan Xie Yanshuo Jin Hui Meng 《Chemistry (Weinheim an der Bergstrasse, Germany)》2019,25(12):3112-3118
A composite of FeOOH nanocubes anchored on carbon ribbons has been synthesized and used as a cathode material for Li/O2 batteries. Fe2+ ion-exchanged resin serves as a precursor for both FeOOH nanocubes and carbon ribbons, which are formed simultaneously. The as-prepared FeOOH cubes are proposed to have a core–shell structure, with FeOOH as the shell and Prussian blue as the core, based on information from XPS, TEM, and EDS mapping. As a cathode material for Li/O2 batteries, FeOOH delivers a specific capacity of 14816 mA h g−1cathode with a cycling stability of 67 cycles over 400 h. The high performance is related to the low overpotential of the oxygen reduction/evolution reaction on FeOOH. The cube structure, the supporting carbon ribbons, and the -OOH moieties all contribute to the low overpotential. The discharge product Li2O2 can be efficiently decomposed in the FeOOH cathode after a charging process, leading to higher cycling stability. Its high activity and stability make FeOOH a good candidate for use in non-aqueous Li/O2 batteries. 相似文献
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Effect of C60 nanoparticles on elasticity of small unilamellar vesicles composed of DPPC bilayers 下载免费PDF全文
The interaction between C60 nanoparticles and biomembranes has been of great interest in researches over the past decades due to their novel applications as well as potential cytotoxicity.In this work,we study the deformation of the small unilamellar vesicles composed of dipalmitoylphosphatidylcholine(DPPC)lipid bilayers infiltrated with C60 nanoparticles of different molecular concentrations through coarse-grained molecular dynamics simulations.By employing the Helfrich spontaneous curvature model,the bending modulus and the spontaneous curvature of the vesicles with C60 nanoparticles of different concentrations are obtained according to the simulation data.The results show that the bending modulus and the spontaneous curvature of pure DPPC vesicle membranes are approximately 1.6×10^-19J and 1.4 nm^-1,respectively.Both of them increase linearly approximately as the C60 concentration increases from 0 to 16.3%.The density profiles of vesicles,the order of lipid packing and the diffusion characteristics of DPPC and C60 are also investigated. 相似文献
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Dr. Li Xu Xiang Chen Jingheng Wu Jinquan Wang Prof. Liangnian Ji Prof. Dr. Hui Chao 《Chemistry (Weinheim an der Bergstrasse, Germany)》2015,21(10):4008-4020
A series of dinuclear ruthenium(II) complexes were synthesised, and the complexes were determined to be new highly selective compounds for binding to telomeric G‐quadruplex DNA. The interactions of these complexes with telomeric G‐quadruplex DNA were studied by using circular dichroism (CD) spectroscopy, fluorescence resonance energy transfer (FRET) melting assays, isothermal titration calorimetry (ITC) and molecular modelling. The results showed that the complexes 1 , 2 and 4 induced and stabilised the formation of antiparallel G‐quadruplexes of telomeric DNA in the absence of salt or in the presence of 100 mM K+‐containing buffer. Furthermore, complexes 1 and 2 strongly bind to and effectively stabilise the telomeric G‐quadruplex structure and have significant selectivity for G‐quadruplex over duplex DNA. In comparison, complex 3 had a much lesser effect on the G‐quadruplex, suggesting that possession of a suitably sized plane for good π–π stacking with the G‐quadruplets is essential for the interaction of the dinuclear ruthenium(II) complexes with the G‐quadruplex. Moreover, telomerase inhibition by the four complexes and their cellular effects were studied, and complex 1 was determined to be the most promising inhibitor of both telomerase and HeLa cell proliferation. 相似文献
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